Book review     

Emile A. Okal  Jeremy Bloxham  Barry Parsons  Leszek Czechowski  L. Czechowski  S. J. Gibowicz  Ursula B. Marvin  Richard Barakat  Jan Błęcki  Roberto Legnani  Stephen Warren 《Pure and Applied Geophysics》1988,127(1):161-180

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Natural and anthropogenic radionuclide distributions in the northwest Atlantic Ocean   总被引：1，自引：0，他引：1  

J. Kirk Cochran  Hugh D. Livingston  David J. Hirschberg  Lolita D. Surprenant 《Earth and Planetary Science Letters》1987,84(2-3)

We have used in-situ pumps which filter large volumes of sea water through a 1 μm cartridge prefilter and two MnO₂-coated cartridges to obtain information on dissolved and particulate radionuclide distributions in the oceans. Two sites in the northwest Atlantic show subsurface maxima of the fallout radionuclides¹³⁷Cs,^239,240Pu and²⁴¹Am. Although the processes of scavenging onto sinking particles and release at depth may contribute to the tracer distributions, comparison of predicted and measured water column inventories suggests that at least 35–50% of the Pu and²⁴¹Am are supplied to the deep water by advection.The depth distributions of the naturally occurring radionuclides²³²Th,²²⁸Th and²³⁰Th reflect their sources to the oceans.²³²Th shows high dissolved concentrations in surface waters, presumably as a result of atmospheric or riverine supply. Activities of²³²Th decrease with depth to values 0.01 dpm/1000 l.²²⁸Th shows high activities in near surface and near bottom water, due to the distribution of its parent,²²⁸Ra. Dissolved²³⁰Th, produced throughout the water column from²³⁴U decay, increases with depth to 3000 m. Values in the deep water (> 3000 m) are nearly constant ( 0.6–0.7 dpm/1000 l), and the distribution of this tracer (and perhaps other long-lived particle-reactive tracers as well) may be affected by the advection inferred from Pu and²⁴¹Am data.The ratio of particulate to dissolved activity for both²³⁰Th and²²⁸Th is 0.15–0.20. This similarity precludes the calculation of sorption rate constants using a simple model of reversible sorption equilibrium. Moreover, in mid-depths²²⁸Th tends to have a higher particulate/dissolved ratio than²³⁰Th, suggesting uptake and release of²³⁰Th and²²⁸Th by different processes. This could occur if²²⁸Th, produced in surface water, were incorporated into biogenic particles formed there and released as those particles dissolved or decomposed during sinking.²³⁰Th, produced throughout the water column, may more closely approach a sorption equilibrium at all depths.²³⁰Th,²⁴¹Am and^239,240Pu are partitioned onto particles in the sequence Th > Am > Pu with 15% of the²³⁰Th on particles compared with 7% for Am and 1% for Pu. Distribution coefficients (K_d) are 1.3–1.6 × 10⁷ for Th, 5–6 × 10⁶ for Am and 7–10 × 10⁵ for Pu. The lower reactivity for Pu is consistent with analyses of Pu oxidation states which show 85% oxidized (V + VI) Pu. However, theK_d value for Pu may be an upper limit because Pu, like²²⁸Th, may be incorporated into particles in surface waters and released at depth only by destruction of the carrier phase.  相似文献   

Particle mixing rates in sediments of the eastern equatorial Pacific: Evidence from ²¹⁰Pb, ^239,240Pu and ¹³⁷Cs distributions at MANOP sites     

J.Kirk Cochran 《Geochimica et cosmochimica acta》1985,49(5):1195-1210

Particle mixing rates (D_B) calculated from excess ²¹⁰Pb gradients in sediments of the east equatorial Pacific range from 0.04 to 0.5 cm²/y, with variation of a factor of 3–4 at a single site. Diffusion of the ²³⁶Ra daughter ²²²Rn may affect ²¹⁰Pb distributions under conditions of slow mixing and low ²¹⁰Pb flux to the seafloor, as shown by a siliceous ooze-clay core which contained the fallout radionuclides ^239,240Pu and ¹³⁷Cs but no excess ²¹⁰Pb (relative to ²²⁶Ra). There is no clear relationship between ²¹⁰Pbderived mixing rates and sediment type, accumulation rate or organic carbon flux to the sediments. Comparison of ²¹⁰Pb mixing rates with those calculated from ^239,240Pu and ¹³⁷Cs distributions reveals better agreement for a pulse input of the fallout radionuclides (D_B = 0.03?0.4 cm²/y) than for continuous input at a constant rate (D_B = 0.1?1.6 cm²/y), although the Pu and ¹³⁷Cs data are better fit by the latter model. The agreement may be fortuitous because ^239,240Pu and ¹³⁷Cs appear significantly deeper than ²¹⁰Pb in at least one core. Tracer separation could be caused by particle size-selective mixing by the benthic fauna or by chemical mobilization. If the fallout radionuclides are scavenged from surface waters by large, organic-rich particles such as fecal pellets, their release and migration may result from decomposition of the carrier in surface sediments. Either a relatively unreactive form of Pu (e.g. oxidized Pu) has been released by this process or a one-dimensional model is inadequate to explain its observed penetration into the sediments. Activity ratios of ${}^{\mathrm{239,240}}\text{Pu}{}^{137}\text{Cs}$ in the sediments decrease with increasing north latitude, and the trend reflects higher fluxes of ^239,240Pu near the weapons test site at Christmas Island (2°N). The ${}^{\mathrm{239,240}}\text{Pu}{}^{137}\text{Cs}$ ratios and fluxes to the sediment (assuming constant input) at the siliceous ooze-red clay site are consistent with published sediment trap data from a nearby site. Thus if fallout radionuclide fluxes to the sea floor were higher in the past, both ^239,240Pu and ¹³⁷Cs have been released from sinking particles.  相似文献   

Laboratory studies of the diagenesis and mobility of ^239,240pu and ¹³⁷Cs in nearshore sediments     

Edward R. Sholkovitz  J.Kirk Cochran  Anne E. Carey 《Geochimica et cosmochimica acta》1983,47(8):1369-1379

Controlled laboratory experiments have been used to study the diagenetic chemistry of ^239,240Pu ¹³⁷Cs, and ⁵⁵Fe. Experiments using Buzzards Bay sediments in small tanks show that sulfate reduction is accompanied by the production of large pore water concentration gradients of alkalinity, phosphate, ammonia and dissolved organic carbon and the formation of subsurface maxima in Fe and Mn. These pore water profiles demonstrate that bacterially-mediated processes of organic matter degradation and redox reactions can be simulated in the laboratory.A vertical profile of ⁵⁵Fe in pore waters is reported for the first time: it follows the profile of stable Fe and as such has a large (200 dpm/100 kg) subsurface maximum between 2–4 cm depth. Comparison of ⁵⁵Fe/Fe ratios in sediments and pore waters shows that there is preferential solubilization of ⁵⁵Fe over stable Fe.The pore water activities of ^239,240Pu show no gradients within the large uncertainties of the counting statistics, but are two to four times higher than Buzzards Bay seawater (0.05 dpm/100 kg).The activity of ¹³⁷Cs in the pore water profile is constant (40 dpm/100 kg) within the large counting uncertainties and is twice that of Buzzards Bay seawater. Cs-137 does not appear to be involved in diagenetic chemistry but may increase in pore waters as a result of ion exchange reactions.Flux estimates based on the pore water data show that remobilization and transport of ^239,240 Pu in coastal sediments are not significant processes while the transport of ^l37Cs may be.  相似文献   

The Boulder     

Ursula B. Marvin 《Earth, Moon, and Planets》1975,14(3-4):315-326

The external morphologies of Boulder 1, Station 2, and of the four samples taken from it by the Apollo 17 crew, are briefly described. The boulder is a polymict breccia, containing the following principal materials as clasts: gray competent breccias (GCBx), black competent breccias (BCBx), anorthositic breccias (AnBx), pigeonite basalt (PB), coarse norite (CN). All are enclosed in a matrix of light-colored friable breccia (LFBx).  相似文献   

New calibration data for the Fe–Ti oxide thermo-oxybarometers from experiments in the Fe–Ti–O system at 1 bar, 1,000–1,300°C and a large range of oxygen fugacities     

Dominique?LattardEmail author  Ursula?Sauerzapf  Martin?K?semann 《Contributions to Mineralogy and Petrology》2005,149(6):735-754

The current formulations of the Fe–Ti oxide thermobarometer (titanomagnetite–ilmenite_ss) fail to reproduce experimental results, in particular at the high temperatures that are relevant for basaltic assemblages. With the aim of improving the experimental basis of the calibration in the Fe–Ti–O system, we have synthesised assemblages of titanomagnetite–ilmenite_ss (Tmt–Ilm_ss), ilmenite_ss–pseudobrookite_ss (Ilm_ss–Psb_ss) and single-phase samples under a wide range of fO₂ (fixed with CO/CO₂ mixtures or by solid oxygen buffers) in sub-solidus conditions (1,000–1,300°C) at 1 bar. Runs lasted 24 h at 1,300°C and up to 240 h at 1,000°C and were terminated by quenching in water. All run products are polycrystalline, roughly equigranular aggregates, with grain sizes of 10–50 m. They were examined and analysed with the SEM and EMP. Tmt compositions are broadly in accordance with the current models at moderate fO₂, but significantly richer in Ti at low fO₂ and high T, due to cationic vacancies. Ilm_ss compositions depart from the predicted values practically at all fO₂ and T conditions, which is related to unsatisfactory thermodynamic models for the rhombohedral oxide. For Ilm_ss–Psb_ss assemblages the best agreement between our data and current calculations is at 1,000°C and moderately high fO₂. Otherwise, experimental and calculated data strongly disagree. The experimental data set on the three Fe–Ti oxide solid solutions presented here is intended to support new versions of both the titanomagnetite–ilmenite_ss thermo-oxybarometer and the ilmenite_ss–pseudobrookite_ss oxybarometer.  相似文献   

Chemical Flux Associated with Spatially and Temporally Variable Submarine Groundwater Discharge,and Chemical Modification in the Subterranean Estuary at Gloucester Point,VA (USA)     

Aaron J. Beck  Alex A. Kellum  Jenna L. Luek  Michele A. Cochran 《Estuaries and Coasts》2016,39(1):1-12

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Tropical Storm Gamma and the Mosquitia of eastern Honduras: a little-known story from the 2005 hurricane season     

David M Cochran Jr  Carl A Reese  Kam-biu Liu 《Area》2009,41(4):425-434

The 2005 Atlantic hurricane season was unprecedented in terms of storm activity in the United States, Mexico, Central America and Caribbean. Given the impacts of hurricanes Katrina and Rita, the Honduran Mosquitia sparked little attention despite being hit by two hurricanes and a tropical storm in 2005. This article recounts the history of these storms in the Afro-Caribbean community of Batalla, drawing from public weather advisories and testimony of local residents obtained through participatory research. We contextualise this local history with results from the first paleotempestological study undertaken in the Mosquitia to shed light on long-term risk of catastrophic storms in the region and to demonstrate the value of integrating these two research approaches. Our findings contribute to recent ethnographic research on hazards by describing how a coastal people understand and respond to tropical cyclones and how landscape change influences the vulnerability of a coastal area. Although residents have not witnessed a storm as intense as those documented in the paleotempestological record, their knowledge and perceptions show how tropical cyclones can be disasters while leaving behind no sedimentary records. The paleotempestological evidence, however, reminds us that catastrophic hurricanes have struck the Mosquitia in the past and will do so again in the future. Understanding the interactions between contemporary human perceptions and responses and long-term hurricane risk provides insight for emergency managers and local stakeholders to better prepare for such a catastrophic event.  相似文献   

A dense bottom water plume in the western Barents Sea: downstream modification and interannual variability     

Ursula Schauer  Eberhard Fahrbach 《Deep Sea Research Part I: Oceanographic Research Papers》1999,46(12):401

The generation and downstream modification of a cold dense Arctic shelf water plume were studied with moored current meters, thermistor chains and conductivity/temperature sensors deployed from August 1993 to September 1994 south of the Storfjord in the Svalbard Archipelago. These observations are compared to similar time series from 1991/92. In 1993/94, bottom water with temperatures close to the freezing point drained continuously from Storfjord between March and September with a mean speed of 0.14 m s⁻¹. About 1.5 months after the plume front had left the Storfjord, it reached the shelf break, 150 km away. The plume had increased its width from 15 km to about 35 km, but its thickness of 50 m remained almost constant and it left the shelf edge at a similar speed. The increased volume transport and the change of temperature/salinity properties indicate an entrainment of 110% of ambient Atlantic water into the plume on its way from the production area to the shelf edge.The maximum salinity of the cold plume was 0.2 lower in 1993/94 than in 1991/92, whilst the temperature/salinity-range of the surrounding Atlantic water remained unchanged. Probably as a dynamic consequence, the speed of the plume was considerably lower in 1993/94. The lower salinity of the plume in 1993/94 is a result of both the 30% less ice formation in Storfjord, caused by lower heat flux and less open water, and a lower surface salinity at the beginning of ice formation. During 1993/94, the Storfjord plume was too light to sink below 700 m.  相似文献   

Fluvial stacking due to plate collision and uplift during the Early Pleistocene in Cyprus     

Wolfgang Schirmer  Josef Weber  Valerian Bachtadse  Marcelle BouDagher-Fadel  Friedrich Heller  Frank Lehmkuhl  Ioannis Panayides  Ursula Schirmer 《Central European Journal of Geosciences》2010,2(4):514-523

Southern Cyprus is situated within a mosaic terrane that has been fragmented between the northward drifting African and Arabian plates and the Eurasian plate. Enormous uplift of the earth mantle in the Tróodos Mountains is explained by two models. The subduction model explains subduction along the Cyprean arc to be the driving force for uplift whereas after the restraining bend model westward squeezing of Cyprus along strike-slip faulting is responsible for the enormous uplift at restraining bends. Since its emergence as an island in early Miocene times, landscape formation on Cyprus has been strongly controlled by this uplift. Until the Plio-Pleistocene, a strait belt separated the southern unroofed ophiolitic core region-the Tróodos Mountains-from the folded Kyrenia range to the north. This former sea basin, nowadays the Mesaoría Basin, is linked with the Tróodos Mountains by a dissected glacis with a thick cover of river deposits. The highest and oldest river deposits (Apalós Formation) were studied in the Vlokkariá hill southwest of Lefkosía. The 45.5 m thick Apalós Formation of Early Pleistocene age exhibits 24 sedimentary units (Fluviatile Series). Their magnetostratigraphical characters align with the Matuyama chron including the Olduvai and Jaramillo subchrons thus comprising about 1.15 Ma within the Early Pleistocene. This fluvial stack indicates a very flat and deeply lying river environment flowing from a slowly uplifting Tróodos hinterland. It happened during the end of Early Pleistocene when the enhanced Tróodos uplift started the dissection of the stacked river plain.  相似文献